Degradation-Aligned Self-Supervised Learning for State of Health Estimation of Lithium-Ion Batteries under Label Sparsity

An accurate estimation of the state of health (SOH) underpins a safe and optimized use of the battery system. Although compelling, data-driven SOH estimation models typically require large amounts of high-quality labeled cycling data, while in practice such labels are often sparse in both quantity and coverage. Therefore, in this work, we propose a degradation-aligned self-supervised learning (SSL) framework based on a convolutional neural network-gated recurrent unit (CNN-GRU) model, which learns aging-consistent representations from unlabeled data through a cycle-order ranking objective as the pretext task for pretraining, thereby enabling robust SOH estimation after fine-tuning on sparsely labeled data. Test results showcase that the proposed ranking-based SSL approach proves to endow the pretrained model with degradation-aligned information from unlabeled data, and after fine-tuning the model can carry out accurate, robust SOH estimation, even when only an extremely limited amount of 1% of unevenly distributed labeled training data is available, where the MAE of 1.718% and RMSE of 2.329% can be achieved on the test cell. In addition, in-depth analyses are presented regarding the influences of label distribution of battery degradation data. We believe this work could shed new light on SOH estimation of lithium-ion batteries under label sparsity in real-world applications.

AI-Driven Surrogate Models for Predicting Electrode-Scale Discharge Behavior in Lithium-Ion Batteries

Physics-based simulations are essential for understanding the electrode-scale discharge behavior of lithium-ion batteries (LIBs) but suffer from prohibitive computational costs. To address this, we introduce a novel deep learning surrogate pipeline based on the Swin3D Transformer to predict spatiotemporal discharge dynamics directly from volumetric data. Our approach integrates two key innovations: Gaussian Positional Encoding (GPE), which enhances spatial feature representation by adapting to the complex geometry of electrode microstructures, and a specialized Temporal Encoding module to capture non-linear timeseries evolution. Experimental validation on an Electrochemical Simulation (ES) dataset demonstrates that our pipeline significantly outperforms state-of-the-art point cloud baselines in prediction accuracy. Furthermore, the proposed method reduces the computational overhead by orders of magnitude, providing a scalable and efficient framework for high-throughput battery design and optimization.

Bridging battery design and health assessment through virtual sensing and physics-informed learning

Supercharging of lithium-ion batteries (LiBs) requires robust health monitoring to ensure durability, safety, and user confidence, particularly for emerging vehicle-to-grid applications with bidirectional energy flows. Yet battery management remains largely disconnected from the material and structural origins of aging, limiting both interpretable health assessment and informed battery design. Here we propose a physics-informed learning framework with virtual sensing that infers hard-to-measure design parameters, including solid-state diffusion coefficient, electrode thickness, ion concentration, and particle size, directly from standard battery management system (BMS) measurements. Across diverse fast-charging strategies and driving profiles, embedding a digital-twin-derived particle-cracking mechanism as a soft constraint reduces trajectory and lifetime prediction errors by 6-8 times relative to state-of-the-art machine learning baselines using only 2% early-life observations. We further show that accurate degradation extrapolation does not require fully resolved governing equations; validated partial mechanisms, jointly refined with limited data, provide sufficient guidance. Virtual sensing transforms standard charging signals into latent design variables without additional sensors, bridging observable battery behavior and underlying aging processes while reducing capacity loss error by up to 39%, end-of-life (EOL) error by 17%, and prediction variability by up to 54%, enabling real-time exploration of new battery configurations. More broadly, the proposed framework establishes a practical feedback loop between deployment and development, demonstrating how real-world operation can continuously inform upstream design decisions across complex multiphysics systems.

Physics-Informed Neural Network with Transfer Learning for State Estimation in Lithium-Ion Batteries using the Single Particle Model with Electrolyte

Physics-informed neural networks (PINNs) have emerged as a powerful tool for solving nonlinear partial differential equations (PDEs), including battery electrochemical models. They typically en-force conservation laws within the loss function to ensure physically consistent solutions. Tradi-tional numerical methods such as finite difference, finite volume, and finite element techniques, re-ly on discretization and can be computationally expensive for nonlinear systems. To address this challenge, PINNs offer improved scalability, particularly for reduced-order models like the single particle model with electrolyte (SPMe). The SPMe describes lithium-ion battery dynamics through coupled diffusion, transport, reaction kinetics, and voltage equations. Despite these advantages, training SPMe-based PINNs from scratch for different battery chemistries or operating conditions is demanding and often leads to slow convergence. To overcome this limitation, this work introduces a transfer learning framework for SPMe-PINNs. The model is first pretrained to learn general elec-trochemical dynamics and then adapted to a target battery by transferring weights, freezing se-lected layers, and fine tuning the remaining parameters, including estimating key electrochemical variables. Validation using PyBaMM demonstrates accurate voltage prediction, indicating that the proposed approach preserves electrochemical consistency while reducing training time and ena-bling efficient generalization across batteries.